Magdalena Marganska-Lyzniak

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magdalena [dot] marganska [at] ur [dot] de


+49 (0)941 943 2042


Institute for Theoretical Physics in Regensburg



Metallic carbon nanotube quantum dots with broken symmetries as a platform for tunable terahertz detection


Journal article


Gilles Buchs, Magdalena Marganska, Jhon González, Kristjan Eimre, Carlo Pignedoli, Daniele Passerone, A. Ayuela, Oliver Gröning, Dario Bercioux
Applied Physics Reviews, vol. 8, 2021 May, p. 021406


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APA   Click to copy
Buchs, G., Marganska, M., González, J., Eimre, K., Pignedoli, C., Passerone, D., … Bercioux, D. (2021). Metallic carbon nanotube quantum dots with broken symmetries as a platform for tunable terahertz detection. Applied Physics Reviews, 8, 021406. https://doi.org/10.1063/5.0018944


Chicago/Turabian   Click to copy
Buchs, Gilles, Magdalena Marganska, Jhon González, Kristjan Eimre, Carlo Pignedoli, Daniele Passerone, A. Ayuela, Oliver Gröning, and Dario Bercioux. “Metallic Carbon Nanotube Quantum Dots with Broken Symmetries as a Platform for Tunable Terahertz Detection.” Applied Physics Reviews 8 (May 2021): 021406.


MLA   Click to copy
Buchs, Gilles, et al. “Metallic Carbon Nanotube Quantum Dots with Broken Symmetries as a Platform for Tunable Terahertz Detection.” Applied Physics Reviews, vol. 8, May 2021, p. 021406, doi:10.1063/5.0018944.


BibTeX   Click to copy

@article{buchs2021a,
  title = {Metallic carbon nanotube quantum dots with broken symmetries as a platform for tunable terahertz detection},
  year = {2021},
  month = may,
  journal = {Applied Physics Reviews},
  pages = {021406},
  volume = {8},
  doi = {10.1063/5.0018944},
  author = {Buchs, Gilles and Marganska, Magdalena and González, Jhon and Eimre, Kristjan and Pignedoli, Carlo and Passerone, Daniele and Ayuela, A. and Gröning, Oliver and Bercioux, Dario},
  month_numeric = {5}
}

Abstract

Generating and detecting radiation in the technologically relevant range of the so-called terahertz gap (0.1–10 THz) is challenging because of a lack of efficient sources and detectors. Quantum dots in carbon nanotubes have shown great potential to build sensitive terahertz detectors, usually based on photon-assisted tunneling. A recently reported mechanism combining resonant quantum dot transitions and tunneling barrier asymmetries results in a narrow linewidth photocurrent response with a large signal-to-noise ratio under weak THz radiation. That device was sensitive to one frequency, corresponding to transitions between equidistant quantized states. In this work we show, using numerical simulations together with scanning tunneling spectroscopy studies of a defect-induced metallic zigzag single-walled carbon nanotubequantum dot, that breaking simultaneously various symmetries in metallic nanotube quantum dots of arbitrary chirality strongly relaxes the selection rules in the electric dipole approximation and removes energy degeneracies. This leads to a richer set of allowed optical transitionsspanning frequencies from 1 THz to several tens of THz, for a ~10 nm quantum dot. Based on these findings, we propose a terahertz detector device based on a metallic single-walled carbon nanotube quantum dot defined by artificial defects. Depending on its length and contacts transparency, the operating regimes range from a high-resolution gate-tunable terahertz sensor to a broadband terahertz detector. Our calculations indicate that the device is largely unaffected by temperatures up to 100 K, making carbon nanotube quantum dots with broken symmetries a promising platform to design tunable terahertz detectors that could operate at liquid nitrogen temperatures.





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